J. H. Oh, H. W. Lee, S. Mannsfeld, R. M. Stoltenberg, E. Jung, Y. W. Jin, J. M. Kim, J.-B. Yoo, Z. Bao, “Solution-Processed, High-Performance n-Channel Organic Microwire Transistors”, Proc. Natl. Acad. Sci. USA 2009, 106, 6065–6070.
[Featured from the cover] [Highlighted in the following media]
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The development of solution-processable, high-performance n-channel organic semiconductors is crucial to realizing low-cost, all-organic complementary circuits. Single-crystalline organic semiconductor nano/microwires (NWs/MWs) have great potential as active materials in solution-formed high-performance transistors. However, the technology to integrate these elements into functional networks with controlled alignment and density lags far behind their inorganic counterparts. Here, we report a solution-processing approach to achieve high-performance air-stable n-channel organic transistors (the field-effect mobility (μ) up to 0.24 cm2/Vs for MW networks) comprising high mobility, solution-synthesized single-crystalline organic semiconducting MWs (μ as high as 1.4 cm2/Vs for individual MWs) and a filtration-and-transfer (FAT) alignment method. The FAT method enables facile control over both alignment and density of MWs. Our approach presents a route toward solution-processed, high-performance organic transistors and could be used for directed assembly of various functional organic and inorganic NWs/MWs.
* Full paper about it → http://www.pnas.org/content/106/15/6065